Everything else is simpler. You don't have to count fields to figure out whether you're dealing with a day vs a month, or an hour vs minute, no matter how the fields are aligned or how long or complex they are. You can scan left and right and look for space and dash and colon to figure out where you are. The formats for time and date are distinctive and ubiquitous. You don't have to guess what you're looking at when you just see one of them in isolation.
Very little follows from cron's format. You have to learn which fields are which for your particular implementation: does it include seconds? You have to learn the bizarre interaction between day and weekday, to do something non-trivial with them. You have to carefully keep track of which field you're in because you can't determine that from neighboring syntax. The visual clutter, if you want to call it that, of systemd's iso8601-based syntax only applies if you're doing complicated rules. In the vast majority of cases it would simply be an ISO8601 timestamp with various values replaced with *'s, and at most one /.
That first impression you had is what I thought too, before diving into it for my previous replies. But no, cron logic is that day and weekday are ORed. It lets you do clever things like run a script on the 1st and 15th of every month, AND on mondays, all in one line. I don't think I've ever seen such a thing in the wild. I'd go so far as to say it's stupid, because it's likely to be misinterpreted if anyone did use it that way. All the other fields are ANDed. I would say that systemd's AND logic is better... and more consistent, which is your own acceptance criterion.