The ADC example in the README is pretty fun; being able to stream data out to a PC at a high rate over a standard interface is always useful in some niche use case, and I don't think anyone has managed High Speed USB over PIO (yet?) so this is likely to be the fastest way.
Combined with RMII ethernet phys only costing around 30 cents even at single quantities definitely makes it just a fun project, though definitely an impressive one at that.