Fixing an existing repository requires a full repack, and for a repository as big as Chromium it still takes more than half a day (56000 seconds is 15h30), even if that's an improvement over the previous 3 days it's a lot of compute.
From my experience of previous attempts, trying to get Github to run a full repack with harsh settings is extremely difficult (possibly because their infrastructure relies on more loosely packed repositories), I tried to get that for $dayjob's primary repository whose initial checkout had gotten pretty large and got nowhere.
As of right now, said repository is ~9.5GB on disk on initial clone (full, not partial, excluding working copy). Locally running `repack -adf --window 250` brings it down to ~1.5GB, at the cost of a few hours of CPU.
The repository does have some of the attributes described in TFA, so I'm definitely looking forward to trying these changes out.