Fwiw this was some years ago and we moved most of our stuff away from them in response. I didn't get the feeling that this was malicious from their side, more like growing pains / mediocre support people / etc. But the end result was the same as you describe, except we chose not to pay up.
EDIT: more context: I shared this story on HN once before, jgrahamc responded with “please email me”, we did but it didn't move the needle. This further convinced me that CF just has a lot of stuff going on and something weird about our traffic made them error out. My suspicion is that the enterprise plan was supposed to make it internally defensible to pour more engineering resources into our case, but they were never explicit about that which made us worry enough to not do it.
I think that a large reputable business like CF should be clearer about stuff like this. That said, as someone running an API business, I also hold some sympathy for “customer does something weird an unexpected, it’s hitting a limit we didn't even know we had, srsly now what?”. The answer to that should be “work together with the customer to get to the bottom of things, customer might need to make changes too”. They didn't do that, which disappointed us, but I can relate to the situation nonetheless.
We’re still a CF customer, just not for this part of our offering.