At least, I couldn't figure out how to do it with IPv6 (no (need for) NAT) - I ended up dropping them if not destined for my desired DNS instead.
(NAT lets you Translate Addresses, usually to save IPv4 space, but here to redirect to a different DNS. IPv6 fixes the address space problem with more addresses, so the hack is done away with, and everything on the network can 'route itself' to everything else without any translation, as pre-NAT and as always intended.)